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Enhancing the performance of silicon-based anode materials for

This has led to growing interest in sodium-ion batteries (SIBs) and potassium-ion batteries (PIBs) as viable alternatives to LIBs. Batteries based on these alkali metals (Li, Na,

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Atom-Level Understanding of the Sodiation Process in Silicon

We report an atomic-level study on the applicability of a Si anode in Na ion batteries using ab initio molecular dynamics simulations. While crystalline Si is not suitable for alloying with Na atoms, amorphous Si can accommodate 0.76 Na atoms per Si atom, corresponding to a specific capacity of 725 mA h g –1.

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Advanced Anode Materials for Rechargeable Sodium-Ion Batteries

Rechargeable sodium-ion batteries (SIBs) have been considered as promising energy storage devices owing to the similar "rocking chair" working mechanism as lithium-ion batteries and abundant and low-cost sodium resource. However, the large ionic radius of the Na-ion (1.07 Å) brings a key scientific challenge, restricting the development of electrode

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Synthesis and characterization of crystalline cristobalite alpha low

Silicon dioxide (SiO2 or Silica) is one of the most prevalent substances in the crust of the Earth. The main varieties of crystalline silica are quartz, cristobalite, and tridymite. When applied as a material for energy, it is affordable and eco-friendly. The SiO2 is considered as electrochemically inactive toward lithium. The SiO2 exhibits low activity for diffusion and

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Pomegranate Peel-Derived Hard Carbons as Anode Materials for Sodium-Ion

When used as a sodium ion battery anode, the PPHC-1100 demonstrated a reversible capacity of up to 330 mAh g−1, maintaining 174 mAh g−1 at an increased current rate of 1 C. After 200 cycles at 0.5 C, the capacity delivered by PPHC-1100 was 175 mAh g−1. The electrochemical behavior of PPHC electrodes was investigated, revealing that the PPHC-1100

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First-Principles Study of Sodium Intercalation in Crystalline Na

We show that Na x Si 24 forms a solid solution with minimal volume changes. Yet sodium diffusion is predicted to be insufficiently fast for facile kinetics of Na-ion intake. Considering these...

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Monolithic Layered Silicon Composed of a Crystalline

While nanostructural engineering holds promise for improving the stability of high-capacity silicon (Si) anodes in lithium-ion batteries (LIBs), challenges like complex synthesis and the high cost of nano-Si impede its commercial application. In this study, we present a local reduction technique to synthesize micron-scale monolithic layered Si (10–20 μm) with a high

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A Brief Overview of Silicon Nanoparticles as Anode Material: A

The successful utilization of silicon nanoparticles (Si-NPs) to enhance the performance of Li-ion batteries (LIBs) has demonstrated their potential as high-capacity anode materials for next-generation LIBs. Additionally, the availability and relatively low cost of sodium resources have a significant influence on developing Na-ion batteries

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Recent trending insights for enhancing silicon anode in lithium-ion

Silicon (Si) was initially considered a promising alternative anode material for the next generation of lithium-ion batteries (LIBs) due to its abundance, non-toxic nature, relatively low operational potential, and superior specific capacity compared to the commercial graphite anode. Regrettably, silicon has not been widely adopted in practical applications due to its low

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Experimental Study on Sodiation of Amorphous Silicon for Use as Sodium

Unfortunately, the high theoretical capacity (4200 mA h g-1) of silicon by (de-)alloy mechanism is limited by its severe volume changes (ΔV ~ 200% - 400%) during cycling for lithium-ion batteries

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Dendrite-free Sb-doped NASICON-type Na

4 天之前· Interfacial reactivity benchmarking of the sodium ion conductors Na 3 PS 4 and sodium β-alumina for protected sodium metal anodes and sodium all-solid-state batteries ACS Appl. Mater. Interfaces, 8 ( 2016 ), pp. 28216 - 28224, 10.1021/acsami.6b10119

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Sb-Si Alloys and Multilayers for Sodium Ion Battery Anodes

Silicon has been intensively studied as a Li-ion battery (LIB) anode material because of its high theoretical storage capacity of ~3600 mAh/g1,2. It also has one of the highest theoretical

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Pre-sodiation strategies for constructing high-performance

3 天之前· As a promising energy storage system, sodium-ion batteries (SIBs) have attracted much attention because of the abundant resource of sodium and its relatively low cost.

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First-Principles Study of Sodium Intercalation in Crystalline Na

Forming a solid-state solution of crystalline silicon under electrochemical conditions is one of the best strategies to preserve the morphology of the anode during cycling. Indeed, lithium has been inserted electrochemically into crystalline silicon, with Li

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Pre-sodiation strategies for constructing high-performance sodium-ion

3 天之前· As a promising energy storage system, sodium-ion batteries (SIBs) have attracted much attention because of the abundant resource of sodium and its relatively low cost. However, the low initial Coulombic efficiency and sodium deficiency (continuous sodium-ion loss or sodium-deficient cathodes) of SIBs result in a lo Journal of Materials Chemistry A Recent Review Articles

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Sb–Si Alloys and Multilayers for Sodium-Ion Battery

By combining silicon and antimony, either by cosputtering or depositing multilayers with bilayer thickness down to 2 nm, we can achieve capacities exceeding even the theoretical capacity of Sb (660 mAh/g).

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Constructing long-cycling crystalline C

The development of advanced energy storage technologies is of significance in realizing large-scale utilization of sustainable energy, especially with the recent rising concerns about supply issues of fossil fuels and their environmental problems. 1-4 Different from lithium-ion batteries (LIBs) that need unevenly distributed lithium resources, sodium-ion batteries (SIBs)

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First-Principles Study of Sodium Intercalation in Crystalline Na

Forming a solid-state solution of crystalline silicon under electrochemical conditions is one of the best strategies to preserve the morphology of the anode during cycling. Indeed, lithium has

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Sb–Si Alloys and Multilayers for Sodium-Ion Battery Anodes

By combining silicon and antimony, either by cosputtering or depositing multilayers with bilayer thickness down to 2 nm, we can achieve capacities exceeding even the theoretical capacity of Sb (660 mAh/g).

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Atom-Level Understanding of the Sodiation Process in

We report an atomic-level study on the applicability of a Si anode in Na ion batteries using ab initio molecular dynamics simulations. While crystalline Si is not suitable for alloying with Na atoms, amorphous Si can accommodate 0.76 Na

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Sodium-ion battery from sea salt: a review | Materials for

Oxide-based materials have also been developed as well, as anodes in sodium-ion batteries, such as (NTP), NaTi 2 (PO 4) 3, Na 2 Ti 3 O 7 and its composites with carbon, which have been studied by several researchers [29, 39].The three-dimensional structure of NTP, which creates an open framework of large interstitial spaces modified with NMNCO, with rate

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Dendrite-free Sb-doped NASICON-type Na

4 天之前· Interfacial reactivity benchmarking of the sodium ion conductors Na 3 PS 4 and sodium β-alumina for protected sodium metal anodes and sodium all-solid-state batteries ACS Appl.

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First-Principles Study of Sodium Intercalation in

We show that Na x Si 24 forms a solid solution with minimal volume changes. Yet sodium diffusion is predicted to be insufficiently fast for facile kinetics of Na-ion intake. Considering these...

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A Brief Overview of Silicon Nanoparticles as Anode Material: A

3 Silicon in Sodium-Ion Batteries Similar to LIBs, it has been demonstrated that alloy-type materials possess the highest specific capacity to be used as anode in high-energy SIBs. [ 114 - 116 ] The highest capacity among allying-type materials for SIBs anodes belongs to phosphorus that forms an alloying binary phase of Na 3 P offering an amazing theoretical

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Experimental Study on Sodiation of Amorphous Silicon for Use as Sodium

Sodium has been considered a potential alternative to lithium because of its earth abundance and lower cost [1], [2]. Moreover, sodium has a redox potential that is only 0.3 V above that of lithium, and the operating principle of Na

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Stable sodium-ion battery anode enabled by encapsulating Sb

Antimony (Sb) has been recognized as one of the most promising metal anode materials for sodium-ion batteries, owing to its high capacity and suitable sodiation potential. Nevertheless, the large volume variation during (de)alloying can lead to material fracture and amorphization, which seriously affects their cycling stability. In this work, we report an

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Enhancing the performance of silicon-based anode materials for

This has led to growing interest in sodium-ion batteries (SIBs) and potassium-ion batteries (PIBs) as viable alternatives to LIBs. Batteries based on these alkali metals (Li, Na, K) show a similar "rocking-chair" mechanism, where ions are reversibly exchanged between electrodes through electrolyte, as shown in Fig. 1 c [32], [33] .

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A Brief Overview of Silicon Nanoparticles as Anode

The successful utilization of silicon nanoparticles (Si-NPs) to enhance the performance of Li-ion batteries (LIBs) has demonstrated their potential as high-capacity anode materials for next-generation LIBs. Additionally, the availability

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Sb-Si Alloys and Multilayers for Sodium Ion Battery Anodes

Silicon has been intensively studied as a Li-ion battery (LIB) anode material because of its high theoretical storage capacity of ~3600 mAh/g1,2. It also has one of the highest theoretical reversible capacities for sodium-ion battery (SIB) anodes (954 mAh/g), corresponding to a one-to-one ratio of sodium to silicon (NaSi). Because of the low

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6 FAQs about [Sodium ion for crystalline silicon battery]

Can Si be used in Na ion batteries?

Despite the exceptionally large capacities in Li ion batteries, Si has been considered inappropriate for applications in Na ion batteries. We report an atomic-level study on the applicability of a

Can a Si anode be used in Na ion batteries?

We report an atomic-level study on the applicability of a Si anode in Na ion batteries using ab initio molecular dynamics simulations. While crystalline Si is not suitable for alloying with Na atoms, amorphous Si can accommodate 0.76 Na atoms per Si atom, corresponding to a specific capacity of 725 mA h g –1.

Is silicon a good anode material for alkali metal ion batteries?

Silicon (Si) has emerged as a promising next-generation anode materials in alkali metal (Li, Na, K) ion batteries due to its high theoretical capacity, suitable working voltage, and abundance in the Earth's crust.

Can silicon nanoparticles improve the performance of Li-ion batteries?

The successful utilization of silicon nanoparticles (Si-NPs) to enhance the performance of Li-ion batteries (LIBs) has demonstrated their potential as high-capacity anode materials for next-generation LIBs. Additionally, the availability and relatively low cost of sodium resources have a significant influence on developing Na-ion batteries (SIBs).

Which cathode material is best for Li/Na/K ion batteries?

Finding cathode materials that can match the high capacity and cycling stability of Si anodes is crucial for the overall efficiency and longevity of Li/Na/K ion batteries. The safety of Si-based anodes in alkali metal ion batteries is a paramount concern, primarily due to the significant volume expansion of Si during charge and discharge cycles.

Are Si-based anodes safe in alkali metal ion batteries?

The safety of Si-based anodes in alkali metal ion batteries is a paramount concern, primarily due to the significant volume expansion of Si during charge and discharge cycles. This expansion leads to instability in the SEI layer and subsequent electrolyte decomposition, increasing the risk of lithium dendrite formation.

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